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Because I have plenty on hand at all times, I would use plastic automotive body filler.
Or "Bondo" (that's a brand).

But a hobby store would have some modeling filler putty in a small tube that would be easier to work with, and cheaper by far because you only need a small amount.

Good Luck!
Lum :wave:
 

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I think the smoothing was to fill the tire tread to simulate wear?
If that is what the op wants to do - then an emory board (finger nail file) will take care of tread patterns on the edge of tires and tread depth on the rolling face - very quickly!
 
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